As of the time of this guide's release, there are a total of 3 unique secret units in Anime Origins. They are Valcrad, who is based off of Alucard from Hellsing, Madaro who is essentially just Madara ...
Our Anime Origins tier list is where I'll separate the units that can carry you from the ones that are mostly there to look nice. Though, to be fair, this game has plenty of unique anime characters ...
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